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《中国科学:材料科学》2023年第5期

中国科学材料 中国科学材料 2023-07-03


Cover Story 

A new stable zero-dimensional hybrid piezoelectric material, [Me-V]3-Mn(SCN)5, is reported, which can serve as eco-friendly materials for energyharvesting and flexible sensors. The device assembled with this hybrid materialshows great piezoelectric energy harvesting properties with an outputvoltage of 18.49 V and a power density of 7.88 μW cm-2 under an appliedforce of only 0.03 MPa. Meanwhile, it is demonstrated to exhibit excellentmechanical durability under operation for 5500 cycles and high environmentalstability over 60 days. The device also shows good sensitivity inmonitoring human body motions, including finger tapping, wrist and elbowbending, and foot stepping (see the article on page 1854).


REVIEW

High-entropy alloys in water electrolysis: Recent advances, fundamentals, and challenges

高熵合金在水电解中的研究进展、基础与挑战

Quan Zhang, Kang Lian, Gaocan Qi (齐高璨), Shusheng Zhang, Qian Liu, Yang Luo (罗扬), Jun Luo, Xijun Liu (刘熙俊) 

Sci China Mater, 2023, 66(5): 1681–1701



REVIEW

Recent application progress and key challenges of biomass-derived carbons in resistive strain/pressure sensor

生物质衍生碳在电阻式应变/压力传感器中的最新应用进展与关键挑战

Lu Wu, Xiaoyu Shi, Pratteek Das, Zhong-Shuai Wu (吴忠帅)

Sci China Mater, 2023, 66(5): 1702–1718



ARTICLE

High-performance and mechanically durable semi-transparent organic solar cells with highly transparent active layers

基于透明活性层的高效柔性半透明有机太阳能电池

Yafeng Li, Wei Song (宋伟), Jianqi Zhang, Xiaoli Zhang, Ziyi Ge (葛子义)

Sci China Mater, 2023, 66(5): 1719–1726



ARTICLE

Enhancing hole extraction via carbon nanotubes/poly(3-hexylthiophene) composite for carbon-based CsPbI2Br solar cells with a new record efficiency

碳纳米管/聚三己基噻吩复合材料增强空穴提取助力碳基CsPbI2Br太阳电池实现新的记录效率

Guizhi Zhang, Jianxin Zhang, Zhenxiao Pan, Huashang Rao (饶华商), Xinhua Zhong

Sci China Mater, 2023, 66(5): 1727–1735



ARTICLE

Temperature-dependent synthesis of SnO2 or Sn embedded in hollow porous carbon nanofibers toward customized lithium-ion batteries

温度调控制备锡或二氧化锡@中空多孔碳纳米纤维电极用于个性化定制锂离子电池

Fanghua Liang, Huilong Dong, Zhuyu Ji, Wei Zhang (张伟), Haifeng Zhang, Chunyan Cao (曹春艳), Heng Li, Hongchao Liu, Ke-Qin Zhang, Yuekun Lai, Yuxin Tang (汤育欣)Mingzheng Ge  (葛明政)

Sci China Mater, 2023, 66(5): 1736–1746



ARTICLE

Cobalt-decorated carbon nanotube bottlebrushes for boosting polysulfide conversion in lithium-sulfur batteries

钴修饰碳纳米管瓶刷助力锂硫电池多硫化物转化

Junlong Huang, Kunyi Leng, Zongheng Cen, Ruliang Liu, Youlong Zhu, Shaohong Liu (刘绍鸿), Ruowen Fu, Dingcai Wu (吴丁财) 

Sci China Mater, 2023, 66(5): 1747–1756



ARTICLE

An in situ reduction strategy toward dendrite-free Zn anodes

一种原位还原策略用于构筑无枝晶锌负极

Mengqi Zhou, Zhou Wu, Rui Wang, Guoqiang Sun (孙国强), Shuang-Quan Zang (臧双全)

Sci China Mater, 2023, 66(5): 1757–1766



ARTICLE

Engineering semicoherent interface with O-Fe-Se coordination for boosting the capacity and rate capability of a battery-type supercapacitor anode

具有O-Fe-Se配位键的半共格异质界面工程提高电池型超级电容器阳极的容量和倍率

Jiangnan Song, Ting Liu, Yinna He, Yiwei Wang, Yuxiao Zhang, Alan Meng, Xiangcheng Yuan, Lei Wang, Guicun Li, Jian Zhao (赵健), Zhenjiang Li (李镇江)

Sci China Mater, 2023, 66(5): 1767–1778



ARTICLE

Tough, self-healable, antifreezing and redox-mediated gel polymer electrolyte with three-role K3[Fe(CN)]6 for wearable flexible supercapacitors

可穿戴柔性超级电容器用强韧、自修复、抗冻的三角色铁氰化钾氧化还原凝胶聚合物电解质

Jia Yang, Mengxiao Wang, Tao Chen, Xiang Yu (于翔), Gang Qin  (秦刚), Xiaohan Fang, Xiaoxiang Su, Qiang Chen (陈强)

Sci China Mater, 2023, 66(5): 1779–1792



ARTICLE

Tailoring the electronic structure of ZnCo2O4 by incorporating anions with low electronegativity to improve the water oxidation activity

低电负性阴离子掺杂调控钴酸锌的电子结构以提高析氧反应活性

Bing Xiong, Liangbing Ge, Xueyan Lei, Yangkai Wang, Jiwen Yang, Weiwei Li, Xiaoning Li (李晓宁), Zhenxiang Cheng, Zhengping Fu (傅正平), Yalin Lu (陆亚林)

Sci China Mater, 2023, 66(5): 1793–1800



ARTICLE

Synergistic Cu+/Cu0 on Cu2O-Cu interfaces for efficient and selective C2+ production in electrocatalytic CO2 conversion

Cu2O-Cu界面上的Cu+和Cu0协同促进电催化CO2还原高效和高选择性地生成C2+产物

Shengnan Wang, Dan Wang, Benqiang Tian, Xiangxiang Gao, Lu Han, Yang Zhong, Shuchang Song, Zhili Wang, Yaping Li, Jianing Gui, Marshet G. Sendeku, Ying Zhang (张颖), Yun Kuang (邝允), Xiaoming Sun

Sci China Mater, 2023, 66(5): 1801–1809



ARTICLE

Anchoring palladium nanoparticles on CsPbBr3 perovskite nanocrystals for enhanced photocatalytic CO2 reduction

通过锚定钯纳米颗粒在CsPbBr3钙钛矿纳米晶体上从而增强光催化CO2还原

Hongbin Xiao, Qingkai Qian (钱庆凯), Zhigang Zang (臧志刚)

Sci China Mater, 2023, 66(5): 1810–1819



ARTICLE

Antiperovskite nitride Cu3N nanosheets for efficient electrochemical oxidation of methanol to formate

反钙钛矿结构氮化铜纳米片实现高效电催化甲醇氧化转化为甲酸盐

Lei Zhao, Qijiao Sun, Mao Li, Yafei Zhong, Peiqi Shen, Yunxiang Lin, Kun Xu (徐坤)

Sci China Mater, 2023, 66(5): 1820–1828



ARTICLE

Dual lattice oxygens in amorphous Zr-doped manganese oxide for highly efficient aerobic oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid

含双晶格氧的无定形锆掺杂锰氧化物选择性高效氧化5-羟甲基糠醛为2,5-呋喃二羧酸

Yonglin Wen, Lairan He, Hu Li, Yunhui Han, Yiming Zhang, Zanyong Zhuang (庄赞勇), Yan Yu (于岩)

Sci China Mater, 2023, 66(5): 1829–1836



ARTICLE

Unveiling the latent reactivity of imines on pyridine-functionalized covalent organic frameworks for H2O2 photosynthesis

吡啶功能化的亚胺类共价有机框架材料在光合成H2O2中的潜在活性

Shijian Zhou, Hao Hu, Huikang Hu, Qichao Jiang, Haoran Xie, Changlai Li, Shuying Gao, Yan Kong (孔岩), Yingjie Hu (胡应杰)

Sci China Mater, 2023, 66(5): 1837–1846



ARTICLE

Kinetics-induced orientational morphological evolution of Pd-Sb rhombohedra from regular nanocrystals to distorted ones

动力学诱导的Pd-Sb菱面体定向形貌演变

Mengjun Wang, Linzhe Lü, Qiaorong Jiang, Guang Li, Qiming Hong, Mingmin Wang, Yong Xu (徐勇), Xiaoqing Huang (黄小青)

Sci China Mater, 2023, 66(5): 1847–1853



ARTICLE

A new piezoelectric hybrid metal thiocyanide for energy harvesting and human motion sensing

新型杂化金属硫氰化物压电体用于能量收集和动作传感

Ying Zhao, Lian-Cai An, Kai Li (李凯), Yong-Ji Gong, Tian-Meng Guo, Fei-Fei Gao, Yang Lei, Quanwen Li, Wei Li (李伟), Xian-He Bu

Sci China Mater, 2023, 66(5): 1854–1860



ARTICLE

Silicon solar cell-enabled organic photoelectrochemical transistor optoelectronics

硅太阳能电池供能的有机电化学晶体管光电子器件

Yi-Tong Xu, Cheng Yuan, Bing-Yu Zhou, Zheng Li, Jin Hu, Peng Lin, Wei-Wei Zhao (赵伟伟), Hong-Yuan Chen, Jing-Juan Xu (徐静娟)

Sci China Mater, 2023, 66(5): 1861–1869



ARTICLE

Large-area epitaxial growth of 2D ZrS2(1-x)Se2x semiconductor alloys with fully tunable compositions and bandgaps for optoelectronics全组分/带隙可调的二维ZrS2(1-x)Se2x半导体合金的外延生长及其光电应用Jidong Huang, Yan Tian, Yong Cheng, Xingxing Li (李星星), Siyu Zhang, Ji Jiang, Jingren Chen, Gaokai Wang, Jingzhen Li, Zhigang Yin, Xingwang Zhang (张兴旺)Sci China Mater, 2023, 66(5): 1870–1878



ARTICLE

Multilayer SnS2/few-layer MoS2 heterojunctions with in-situ floating photogate toward high-performance photodetectors and optical imaging application

原位集成光浮栅的多层SnS2/少层MoS2异质结用于高性能光电探测器与光学成像

Huaxin Yi, Hailin Yang, Churong Ma (马楚荣), Yuhang Ma, Qiaojue Ye, Jianting Lu, Wan Wang, Zhaoqiang Zheng, Zexiang Deng (邓泽祥), Yichao Zou, Jiandong Yao (姚健东), Guowei Yang

Sci China Mater, 2023, 66(5): 1879–1890



ARTICLE

Highly stretchable and high-mobility simiconducting nanofibrous blend films for fully stretchable organic transistors

高拉伸高迁移率半导体纳米纤维共混薄膜应用于完全可拉伸有机晶体管

Fuming Wu, Yixuan Liu, Jun Zhang, Xiangxiang Li, Hui Yang (杨辉), Wenping Hu

Sci China Mater, 2023, 66(5): 1891–1898



ARTICLE

Highly sensitive, durable, environmentally tolerant and multimodal composite ionogel-based sensor with an ultrawide response range

高灵敏度, 超宽响应范围, 环境耐受性高的多模式离子凝胶基传感器

Jianfei Tie, Zhiping Mao (毛志平), Linping Zhang, Yi Zhong, Xiaofeng Sui, Hong Xu (徐红)

Sci China Mater, 2023, 66(5): 1899–1910



ARTICLE

One 3D aerogel wearable pressure sensor with ultrahigh sensitivity, wide working range, low detection limit for voice recognition and physiological signal monitoring

具有超高灵敏度、宽工作范围、低检测限的3D气凝胶可穿戴压力传感器用于语音识别和生理信号监测

Chengshuo Shang, Xiangtian He, Xiaodi Li, Zerui Liu, Yuxiang Song, Yulin Zhang, Xu Li, Yong Lu, Xiaokang Ding, Ting Liu (刘婷), Jicai Zhang (张纪才), Fu-Jian Xu (徐福建)

Sci China Mater, 2023, 66(5): 1911–1922



ARTICLE

Highly sensitive and self-healing conductive hydrogels fabricated from cationic cellulose nanofiber-dispersed liquid metal for strain sensors

阳离子纤维素纳米纤维分散液态金属制备高灵敏度和自修复导电水凝胶用于应变传感器

Shihao Wu, Bingyan Wang, Duo Chen, Xiaona Liu, Huili Wang, Zhaoping Song, Dehai Yu, Guodong Li, Shaohua Ge, Wenxia Liu (刘温霞)

Sci China Mater, 2023, 66(5): 1923–1933



ARTICLE

Ultra-stretchable hydrogel thermocouples for intelligent wearables

超拉伸水凝胶热电偶

Yifan Zhao, Xifan Fu, Binghan Liu, Jiantao Sun, Zihan Zhuang, Peihua Yang (杨培华), Junwen Zhong (钟俊文)Kang Liu (刘抗) 

Sci China Mater, 2023, 66(5): 1934–1940



ARTICLE

A composite hydrogel exhibiting stiff response at low-strain regime by repulsion effect of positive/negative Poisson’s ratio

正/负泊松比的排斥效应诱导的复合水凝胶在低应变下的刚性响应

Wei Shi, Jin Huang, Tianxu Zhou, Yichao Xu (许一超), Hao Yan (严昊)Mingjie Liu (刘明杰)

Sci China Mater, 2023, 66(5): 1941–1948



ARTICLE

Reconfigurable photoswitchable multistate fluorescent polymer-based information encryption toolbox

基于可重构光开关多态荧光聚合物的信息加密工具箱

Jiawei Jiang, Peisheng Zhang, Yong Tian, Zhong Lin, Chonghua Zhang, Jiaxi Cui (崔家喜), Jian Chen (陈建), Xudong Chen

Sci China Mater, 2023, 66(5): 1949–1958



ARTICLE

Unique mechanofluoro enhancement effect of an AIEgen containing Tröger’s base and TPE units

一种含Tröger碱单元的AIE分子的独特力致荧光增强行为

Juechen Ni, Qiguang Zang, Haoke Zhang, Jing Zhi Sun (孙景志), Ben Zhong Tang (唐本忠)

Sci China Mater, 2023, 66(5): 1959–1967



ARTICLE

High-quality GaN grown on nitrogen-doped monolayer graphene without an intermediate layer

氮掺杂单层石墨烯上无中间层沉积高质量氮化镓

Danni Chen, Jing Ning (宁静), Dong Wang (王东), Boyu Wang, Jianglin Zhao, Jincheng Zhang, Yue Hao

Sci China Mater, 2023, 66(5): 1968–1977



ARTICLE

High-quality AlGaN epitaxial structures and realization of UVC vertical-cavity surface-emitting lasers

高质量的AlGaN外延结构和UVC垂直腔面发射激光器的实现

Zhongming Zheng, Yukun Wang, Jason Hoo, Shiping Guo (郭世平), Yang Mei, Hao Long, Leiying Ying, Zhiwei Zheng, Baoping Zhang (张保平)

Sci China Mater, 2023, 66(5): 1978–1988



ARTICLE

Engineering charge-transfer interactions for red-emitting SrLa(Sc,Ga)O4:Ce3+ phosphor with improved thermal stability

利用电荷转移工程提高红色SrLa(Sc,Ga)O4:Ce3+荧光粉的热稳定性

Zhiyu Yang, Yifei Zhao, Jumpei Ueda, Maxim S. Molokeev, Mengmeng Shang, Zhiguo Xia (夏志国)

Sci China Mater, 2023, 66(5): 1989–1996



ARTICLE

A silane-based host material with improved electron transport properties for phosphorescent OLEDs with high efficiency and low efficiency roll-off

Jinho Park, Junseop Lim, Jun Yeob Lee

Sci China Mater, 2023, 66(5): 1997–2003



ARTICLE

CsPbBr3@PbBrOH 3D/1D molecular matrix for a high-performance scintillator

三维/一维CsPbBr3@PbBrOH分子矩阵高性能闪烁体

Heng Guo, Yizhi Zhu, Qingxian Zhao, Qingsong Jiang, Yi Ma, Jinping Chen, Lei Song, Zengliang Shi (石增良), Chunxiang Xu (徐春祥)

Sci China Mater, 2023, 66(5): 2004–2012



ARTICLE

2D-3D perovskite memristor with low energy consumption and high stability for neural morphology calculation

用于神经形态学计算的低能耗、高稳定性2D-3D钙钛矿忆阻器

Kaixuan Sun, Qingrui Wang, Long Zhou, Jingjuan Wang, Jingjing Chang, Rui Guo (郭瑞), Beng Kang Tay, Xiaobing Yan (闫小兵)

Sci China Mater, 2023, 66(5): 2013–2022



ARTICLE

Light-/steam-driven polymeric crosslinking with porous multistructure pattern for ultrastable and fast-speed memory

光/蒸气协同构建交联多孔聚合物复合结构基超稳定高速阻变存储器

Chaoyi Ban, Yuhang Yin, Xu Luo, Zhengdong Liu (刘正东), Kang Chen, Minghua Tang, Xuemei Dong, Dengfeng Zhang, Zifan Li, Yueyue Wu, Juqing Liu (刘举庆)Wei Huang (黄维)

Sci China Mater, 2023, 66(5): 2023–2031



ARTICLE

Record-high mobility and extreme magnetoresistance on kagome-lattice in compensated semimetal Ni3In2S2

Kagome晶格补偿型半金属Ni3In2S2创纪录的高迁移率和极大磁电阻现象

Hongwei Fang, Meng Lyu, Hao Su, Jian Yuan, Yiwei Li, Lixuan Xu, Shuai Liu, Liyang Wei, Xinqi Liu, Haifeng Yang, Qi Yao, Meixiao Wang, Yanfeng Guo, Wujun Shi (史武军), Yulin Chen (陈宇林), Enke Liu (刘恩克)Zhongkai Liu (柳仲楷)

Sci China Mater, 2023, 66(5): 2032–2038


ARTICLE

Giant low-field magnetocaloric effect of (Er,Y)Cr2Si2 compounds at ultra-low temperatures

Er-Y-Cr-Si化合物在极低温区的巨低场磁热效应

Lei Xi, Xinqi Zheng (郑新奇), Yawei Gao, Jiawang Xu, Chaofan Liu, Dingsong Wang, Juping Xu, Wen Yin, Shuxian Yang, Baojie Jin, Mengyuan Zhu, Weifeng Xu, Jianxin Shen, Jingyan Zhang, He Huang, Yanfei Wu, Fei Gu, Huiyu Shi, Yixuan Tao, Shouguo Wang (王守国), Baogen Shen

Sci China Mater, 2023, 66(5): 2039–2050



ARTICLE

Enhanced thermoelectric properties and electrical stability for Cu1.8S-based alloys: Entropy engineering and Cu vacancy engineering

Cu1.8S基合金的热电性能和电稳定性增强:熵工程和Cu空位工程

Wei Zhou, Hezhang Li (李和章), Zhihang Shan, Rui Zhang, Shikuo Lu, Jun Pei (裴俊), Zhenhua Ge, Min Zhou, Yuanbing Wang, Boping Zhang (张波萍)

Sci China Mater, 2023, 66(5): 2051–2060



ARTICLE

Strong high-entropy diboride ceramics with oxide impurities at 1800°C

1800°C下具有优异高强度且含氧化物杂质的高熵二硼化物陶瓷

Jie Liu, Qing-Qing Yang, Ji Zou (邹冀), Wei-Min Wang, Xin-Gang Wang (王新刚)Zheng-Yi Fu (傅正义)

Sci China Mater, 2023, 66(5): 2061–2070



ARTICLE

Ultra-robust icephobic coatings with high toughness, strong substrate adhesion and self-healing capability

超耐用疏冰涂层的制备及性能研究

Yizhi Zhuo (卓毅智), Verner Håkonsen, Siqi Liu, Tong Li, Feng Wang, Sihai Luo, Senbo Xiao, Jianying He (何健英), Zhiliang Zhang (张志良)

Sci China Mater, 2023, 66(5): 2071–2078



ARTICLE

Controlled synthesis of highly stable lead-free bismuth halide perovskite nanocrystals: Structures and photophysics

高稳定性铋基钙钛矿纳米晶的可控合成:结构和光物理性质

Huifang Geng, Zhuanzhuan Huang, Huaxiu Geng, Siyu Liu, Maria A Naumova, Raffaele Salvia, Siqi Chen, Junli Wei, Lifu Zhang, Xianshao Zou, Weihua Lin, Xinyi Cai, Mingjian Yuan, Zhenpeng Hu, Xi Shen, Richeng Yu, Kaibo Zheng (郑凯波), Sophie E. Canton, Xuewen Fu (付学文)

Sci China Mater, 2023, 66(5): 2079–2089




ARTICLE

Dynamic artificial cells by swarm nanorobotics and synthetic life chemistry

基于集群纳米机器技术和合成生命化学的动态人工细胞

Xiaowen Cheng, Chen Wang, Dong Liu, Yuting Liao, Bin Wang, Xue Zhang, Hao Zheng, Yuan Lu (卢元)

Sci China Mater, 2023, 66(5): 2090–2099



LETTER

Constructing a molecular crystal actuator from pamoic acid with multilevel enhanced photoluminescence by cocrystallization

共结晶法制备具有多级增强光致发光的双羟萘酸分子晶体驱动器

Wenjie Kuang, Yifu Chen, Bo Jing, Guanlun Sun, Songgu Wu, Junbo Gong (龚俊波)

Sci China Mater, 2023, 66(5): 2100–2104



HIGHLIGHT

Ferroelectricity survives in the sub-nanometer scale

Yiqian Liu, Yuan-Hua Lin

Sci China Mater, 2023, 66(5): 2105–2106



2023年文章目录(点击链接可查看各期目录)

《中国科学:材料科学》2023年第4期《中国科学:材料科学》2023年第3期《中国科学:材料科学》2023年第2期《中国科学:材料科学》2023年第1期
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